Quark
Odo
Garak
Gul Dukat
Kira
Odo
Garak
Gul Dukat
Kira
I agree with the list in the OP exactly.
I would add Kai Winn to that list too, though. 6-way tie for the best of the best IMO. All of them fascinatingly nuanced characters and immaculately played by master actors.
#1 has to be Garak. Andy Robinson did so much with a character that was already wonderfully written. It's almost a shame he wasn't made into a regular as planned in the final season, but we ended up seeing plenty of him, anyway.
The rest are harder to choose.
Gul Dukat was a great character through the episode Waltz, but after that he was a caricature of himself.
Damar was a character I really liked in the end, but it took him a while to become more than window dressing on the show.
Quark was usually great, although he was involved in the occasional bad Ferengi episode (of which most I liked, but there's little to be redeemed in Profit and Lace).
I think both Worf and O'Brien had great character arcs on Deep Space Nine, but since they were imported from The Next Generation, I don't know how you'd classify them.
Jeffery Combs is great in any role. I love the season where he played three characters.
I think its interesting that most of our lists consist many of supporting characters, and not the main cast so much
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