Ok, I'm watching Angel's second episode and I'm already thinking about just going through Buffy at once and then going back to Angel. This is already starting to get overwhelming and now that the shows are established it doesn't really feel like that big of a deal anymore.
...I'm so sorry for changing my mind twice in a period of 24 hours.![]()
It's all good. Do you. Your enjoyment is what matters. If you don't like bingeing them simultaneously, then there's no point in lessening the impact of two great shows by watching them in a manner that sucks all your enjoyment out of them. It should be fun, not feel like a massive chore.
If I did it this way, what are the absolute must episodes to see through each series. For example, I'm not looking for Buffy picks up the phone and it's Angel but Angel doesn't reply type scenes. I'm looking at true crossovers like Pangs and Will You Remember Me. That should keep things to a minimum I think.
Oz has a crossover trip to LA coming up, and then there is Pangs and I Will Remember You for season one. And even Oz's trip to LA is more about the MacGuffin than the character beats.
Season 2 has the flashback crossovers in Darla and Fool For Love. After that, I don't think there is anything you need to worry about until the stuff with Faith and Willow in Buffy season 7 and Angel season 5.
I'm sure that theenglish or OCDGeek can point out anything I may have missed.
The epic four-part crossover This Year's Girl/Who Are You?/Five by Five/Sanctuary from towards the end of Buffy: Season 4/Angel: Season 1 is key too. It also gives you a nice taste of the sort of show Angel became in those final five episodes of its inaugural season.
Five by Five/Sanctuary is pretty much the exact moment Angel went from an anthology series to an epic saga. The series myth arc didn't actually kick off until the two-part season finale a couple episodes later, but Five by Five/Sanctuary set the darker tone, greater moral complexity and richer character interactions that defined the series in the years to come.
If nothing else, it gives you something to whet your appetite for Angel while you finish Buffy's seven year journey. Plus the character interactions between Faith and the gang in Buffy: Season 7 will make way more sense with the added context of Faith's character development in those episodes.
EDIT: Oh, for the record. Here's the actual full-on crossover episodes.
Season 4/Season 1
Buffy: The Harsh Light of Day/Angel: In the Dark
Buffy: Pangs/Angel: I Will Remember You
Buffy: This Year's Girl & Who Are You?/Angel: Five by Five & Sanctuary
Season 5/Season 2
Buffy: Fool for Love (flashbacks)/Angel: Darla (flashbacks)
Season 7/Season 4
We'll cross that bridge when we get there, because it is a lot. And both shows went full-on serialized those seasons due to it being Buffy's definite swan song and Angel's possible swan song, so it's a mite complicated. Circling back to see the Angel portions of the crossover for the first time during you eventual Angel binge might be best.
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