Cardassians, mainly because I think they were the best developed of the lot, as nuanced individuals.
The Dominion, and the Founders in particular, mainly because they were so mysterious and remained so for quite a long time.
I also liked early TNG Borg, before they were completely defanged. That started with First Contact and Voyager conclusively completed the process.
Gul Dukat. For many, many, MANY reasons.
Oh and Michael Eddington - mostly for saying this to Sisko...
"I know you. I was like you once, but then I opened my eyes. Open your eyes, Captain. Why is the Federation so obsessed with the Maquis? We've never harmed you. And yet we're constantly arrested and charged with terrorism. Starships chase us through the Badlands and our supporters are harassed and ridiculed. Why? Because we've left the Federation, and that's the one thing you can't accept. Nobody leaves paradise. Everyone should want to be in the Federation. Hell, you even want the Cardassians to join. You're only sending them replicators because one day they can take their 'rightful place' on the Federation Council. You know, in some ways you're even worse than the Borg. At least they tell you about their plans for assimilation. You're more insidious. You assimilate people and they don't even know it."
changelings. Biggest threat, even bigger than the Borg the Federation every faced.
Danny Glover: Except they all have that same damn haircut.But TNG really made them something special. Proper conniving, rarely would they be seen as trite. Except for NEM where it all feels like rubber stamp checkbox stuff so that everyone can be one big happy galactic family*.
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