After some internal debate, I went with some fun ones- Goldfinger, Goldeneye, and Casino Royale.
My next three picks would have been From Russia with Love, On Her Majesty's Secret Service, and The Spy Who Loved Me.
ETA: Hmm, I accidentally voted for Quantum instead of Casino. D'oh!
Good picks Kelso
Even though Sean Connery is my favorite Bond, my top 3 films are
On Her Majesty's Secret Service, Goldeneye and Casino Royale.